Development of Delayed Gamma-Ray Spectroscopy for Nuclear Material Analysis

Year
2018
Author(s)
Michio Seya - Japan Atomic Energy Agency
Mitsuo Koizumi - Japan Atomic Energy Agency
Douglas C. Rodriguez - Japan Atomic Energy Agency
Fabiana Rossi - Japan Atomic Energy Agency
Kamel Abbas - EC Joint Research Centre, Ispra
Ton Takahashi - Japan Atomic Energy Agency
Bent Pedersen - EC Joint Research Centre, Ispra
Abstract
For the past three years the Japan Atomic Energy Agency (JAEA) and the Joint Research Centre (JRC) of the European Commission have been researching the delayed gamma-ray spectroscopy (DGS) technique for nuclear safeguards. DGS has great potential for high-radioactivity nuclear materials (HRNM), such as spent fuel solutions, since it determines fissile nuclide compositions by correlating the observed time-dependent gamma-ray energy spectrum to the unique fission product (FP) yield of the individual nuclides. Experiments were performed with low-radioactivity nuclear material using both the Pulsed Neutron Interrogation Test Assembly (PUNITA) of JRC and a californium shuffler designed at the JAEA and tested in the PERLA Laboratory of JRC. The data was analyzed using an inverse Monte Carlo method that both determines delayed gamma-ray peak intensity correlations and provides an evaluation of the uncertainty of the measurements. The results were used to verify delayed gamma-ray signatures for varying fissile compositions, total fissile content, and DGS interrogation timing patterns. Future development will focus on measuring HRNM and designing a compact active-interrogation system by evaluating different neutron sources, moderating materials, and detection capabilities. This presentation summarizes the JAEA/JRC DGS program to date and the future direction of this collaborative work. This research was performed under the Japanese MEXT subsidiary funding for nuclear security promotion.