Non-destructive Assay of Spent Nuclear Fuel using Passive Neutron Albedo Reactivity

Year
2010
Author(s)
S. Tobin - Los Alamos National Laboratory
Martyn T. Swinhoe - Los Alamos National Laboratory
H. O. Menlove - Los Alamos Scientific Laboratory
L. G. Evans - Los Alamos National Laboratory
Stephen Croft - Los Alamos National Laboratory
M. A. Schear - Los Alamos National Laboratory
Abstract
Passive Neutron Albedo Reactivity (PNAR) is one of fourteen techniques that has been researched and evaluated to form part of a comprehensive and integrated detection system for the non- destructive assay (NDA) of spent nuclear fuel. PNAR implemented with 3He tubes for neutron detection (PNAR-3He) is the measurement of time correlated neutrons from a spent fuel assembly with and without a Cadmium (Cd) layer surrounding the assembly. PNAR utilizes the self- interrogation of the fuel via reflection of neutrons born in the fuel assembly back in to the fuel assembly. The neutrons originate primarily from spontaneous fission events within the fuel itself (Curium-244) but are amplified by multiplication. The presence and removal of the Cd provides two measurement conditions with different neutron energy spectra and therefore different interrogating neutron characteristics. Cd has a high cross-section of absorption for slow neutrons and therefore greatly reduces the low energy (thermal) neutron fluence rate returning. The ratios of the Singles, Doubles and Triples count rates obtained in each case are known as the Cd ratios, which are related to fissile content. A potential safeguards application for which PNAR-3He is particularly suited is “fingerprinting”. Fingerprinting could function as an alternative to plutonium (Pu) mass determination; providing confidence that material was not diverted during transport between sites. PNAR-3He has six primary NDA signatures: Singles, Doubles and Triples count rates measured with two energy spectra at both shipping and receiving sites. This is to uniquely identify the fuel assembly, and confirm no changes have taken place during transport. Changes may indicate an attempt to divert material for example. Here, the physics of the PNAR-3He concept will be explained, alongside a discussion on the development of a prototypical PNAR-3He instrument using simulation.